Research
| Title： | Removal of ammonia nitrogen, nitrate, and phosphate from aqueous solution using biochar derived from Thalia dealbata Fraser: effect of carbonization temperature |
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| First author： | Zhao, Yuqing; Yang, Hang; Xia, Shibin; Wu, Zhenbin |
| Journal： | ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH |
| Years： | 2022 |
| DOI： | 10.1007/s11356-022-19870-z |
| Abstract： | Thalia dealbata Fraser-derived biochar was prepared at different carbonization temperatures to remove nutrients in aqueous solution. Thermogravimetry/differential thermogravimetry (TG/DTG) was used to analyze the carbonization and decomposition procedure of Thalia dealbata Fraser. X-ray diffraction (XRD), scanning electron microscope (SEM), Fourier transform infrared spectroscopy (FTIR), zeta potential, and N-2 adsorption-desorption isotherms were employed to characterize the prepared biochar. The carbonization temperature obviously effected the physical and chemical properties of biochar. The adsorption efficiency of ammonia (NH4+-N), nitrate (NO3--N), and phosphate (PO43-) adsorption on biochar was tested. Pseudo-first-order kinetic, pseudo-second-order kinetic, and intra-particle diffusion kinetic models were used to fit adsorption kinetic. Langmuir and Freundlich models were used to fit adsorption isotherms. The theoretical adsorption capacity of NH4+-N, NO3--N, and PO43- on biochar was 5.8 mg/g, 3.8 mg/g, and 1.3 mg/g, respectively. This study provides the insights for effect of carbonization temperature on biochar preparation and application. |
